Combine greek yogurt and iced coffee in a large blender and pulse until completely combined, about 1 minute.
Fill the bottom of each popsicle mold with 2 teaspoons of granola. Pour iced coffee mixture into molds to fill half way full. Add another layer of 2 teaspoons of granola. Fill the molds the rest of the way with the iced coffee mixture and top with the remaining granola.
Place popsicle sicks in each mold and place in the freezer for at least 6 hours or overnight.